In Situ Optical Microscopy
Transparent-window battery cells let researchers watch dendrites grow and dissolve in real time under a light microscope, tracking growth rate and shape as charging conditions change. It's the most accessible of these techniques, though anything smaller than the microscope's resolution stays invisible.
- 2014Mechanisms of dendritic growth investigated by in situ light microscopy during electrodeposition and dissolution of lithium
Steiger, J., Kramer, D., & Mönig, R.Journal of Power Sources, 261, 112–119
Uses live light microscopy to work out the mechanics behind dendrite growth during plating and stripping.
- 2016Dendrites and Pits: Untangling the Complex Behavior of Lithium Metal Anodes through Operando Video Microscopy
Wood, K. N., et al.ACS Central Science, 2, 790–801
Operando video microscopy separates dendrite growth from pitting as two distinct failure behaviors on lithium metal anodes.
- 2016Transition of lithium growth mechanisms in liquid electrolytes
Bai, P., Li, J., Brushett, F. R., & Bazant, M. Z.Energy & Environmental Science, 9, 3221–3229
Shows lithium switches from slow, mossy growth to fast, tip-driven dendrites once the electrolyte near the electrode runs out of ions — a key reason fast charging is risky.
- 2017Mechanism of Lithium Metal Penetration through Inorganic Solid Electrolytes
Porz, L., et al.Advanced Energy Materials, 7, 1701003
Watches lithium force its way through cracks and flaws in ceramic electrolytes, challenging the idea that a stiff solid electrolyte alone can stop dendrites.
- 2021Visualizing Lithium Dendrite Formation within Solid-State Electrolytes
Sun, M., et al.ACS Energy Letters
Direct visualization of how dendrites nucleate and spread inside solid-state (not liquid) electrolytes.
- 2022The growth mechanism of lithium dendrites and its coupling to mechanical stress
Becherer, J., Kramer, D., & Mönig, R.Journal of Materials Chemistry A, 10, 5530–5539
Links dendrite growth mechanics to the mechanical stress they generate as they push through the cell.